The BSE benchmark had hit the 81,000-mark for the first time on Thursday.
The NSE Nifty tumbled 269.95 points or 1.09 per cent and ended at 24,530.90 after hitting its fresh record peak of 24,854.80 during the opening bell. During the day, it declined 292.7 points or 1.18 per cent to 24,508.15.
Among the Sensex pack, Tata Steel tumbled over 5 per cent while JSW Steel tanked nearly 5 per cent.
Tata Motors, NTPC, UltraTech Cement, Tech Mahindra, Bajaj Finance, Power Grid, Mahindra & Mahindra, and Reliance Industries were the other major laggards.
Infosys climbed nearly 2 per cent after the IT major reported a 7 per cent rise in consolidated net profit at Rs 6,368 crore in the April-June quarter and raised its growth outlook for the current financial year, signalling an improvement in the IT segment.
ITC, Asian Paints and HCL Technologies were the other gainers.
In Asian markets, Seoul, Tokyo and Hong Kong settled lower while Shanghai ended in the green.
European markets were trading lower.
The US markets ended in negative territory on Thursday.
Global oil benchmark Brent crude declined 0.07 per cent to USD 85.05 a barrel.
Foreign Institutional Investors (FIIs) bought equities worth Rs 5,483.63 crore on Thursday, according to exchange data.
The BSE benchmark Sensex jumped 626.91 points or 0.78 per cent to settle at a fresh closing high of 81,343.46 on Thursday.
The broader Nifty climbed 187.85 points or 0.76 per cent to settle at an all-time closing high of 24,800.85.